Electronic-vibrational spectroscopy: A new probe for structure and function. This project aims to solve a major challenge in ultrafast spectroscopy: to identify and quantify competing reaction pathways in complex photochemical systems. Ultrafast Spectroscopy provides information on excited-state processes of photochemical reactions, however, unravelling heterogeneous systems with competing parallel processes remains difficult. Multidimensional electronic-vibrational spectroscopy, sensitive to el ....Electronic-vibrational spectroscopy: A new probe for structure and function. This project aims to solve a major challenge in ultrafast spectroscopy: to identify and quantify competing reaction pathways in complex photochemical systems. Ultrafast Spectroscopy provides information on excited-state processes of photochemical reactions, however, unravelling heterogeneous systems with competing parallel processes remains difficult. Multidimensional electronic-vibrational spectroscopy, sensitive to electronic dynamics and molecular structure, is expected to overcome this barrier. This new level of detail will profoundly enhance our understanding of energy and chemical conversion in complex systems and will reveal design targets for optimising next-generation light-energy harvesting, conducting, and emitting materials.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE200100279
Funder
Australian Research Council
Funding Amount
$424,198.00
Summary
A nanodiamond voltage sensor: towards real-time, long-term neuronal sensing. This project aims to develop a voltage sensor that may ultimately be used to measure neuronal signals noninvasively in real-time and over hours. The project expects to generate the fundamental science needed to use nanodiamonds for fluorescence-based voltage sensing that can be easily measured using optical microscopy. The expected outcome is a biocompatible sensor that should provide a solution to one of the biggest ch ....A nanodiamond voltage sensor: towards real-time, long-term neuronal sensing. This project aims to develop a voltage sensor that may ultimately be used to measure neuronal signals noninvasively in real-time and over hours. The project expects to generate the fundamental science needed to use nanodiamonds for fluorescence-based voltage sensing that can be easily measured using optical microscopy. The expected outcome is a biocompatible sensor that should provide a solution to one of the biggest challenges in neuroscience; the fast, precise and long-term measurement of neuronal activity. This technology may one day inform our understanding of how the normal brain works and provide major insights into mental health conditions and neurodegenerative diseases.Read moreRead less
Multi-colour ultrashort soft X-ray pulses. This project aims to create multi-colour, ultrashort, highly coherent, bright pulses of soft X-rays based on high-harmonic generation in a table-top multiple-section gas cell. Studying multi-electronic and non-adiabatic processes and other fundamental aspects such as multi-electronic correlations and non-Born-Oppenheimer vibronic couplings in complex molecules is a major challenge in current ultrafast photochemistry research. This project will use multi ....Multi-colour ultrashort soft X-ray pulses. This project aims to create multi-colour, ultrashort, highly coherent, bright pulses of soft X-rays based on high-harmonic generation in a table-top multiple-section gas cell. Studying multi-electronic and non-adiabatic processes and other fundamental aspects such as multi-electronic correlations and non-Born-Oppenheimer vibronic couplings in complex molecules is a major challenge in current ultrafast photochemistry research. This project will use multiple driving pulses with different carrier frequencies to control the spectral properties and time delay of the pulses. It will use the soft X-ray source to develop an ideal platform for studying multi-electronic and non-adiabatic processes, multi-electronic correlations and non-Born-Oppenheimer vibronic couplings in complex molecules. This is expected to advance materials science, paving the way to soft X-ray technologies.Read moreRead less
ARC Centre of Excellence in Optical Microcombs for Breakthrough Science. ARC Centre of Excellence in Optical Microcombs for Breakthrough Science. This Centre aims to explore the society wide transformations that will flow from optical frequency combs - thousands of highly pure light signals precisely spaced across the entire optical spectrum - by leveraging and building upon the latest breakthroughs in physics, materials science and nanofabrication. It expects to generate a wide new base of know ....ARC Centre of Excellence in Optical Microcombs for Breakthrough Science. ARC Centre of Excellence in Optical Microcombs for Breakthrough Science. This Centre aims to explore the society wide transformations that will flow from optical frequency combs - thousands of highly pure light signals precisely spaced across the entire optical spectrum - by leveraging and building upon the latest breakthroughs in physics, materials science and nanofabrication. It expects to generate a wide new base of knowledge in fields as diverse as astronomy, spectroscopy, chemical sensors, and precision measurement. Expected outcomes include the capability to realise complete comb systems on a chip the size of a fingernail, tailored to specific applications, with significant benefits spanning from imaging live cells to autonomous vehicles, satellite communications, and the search for exoplanets.Read moreRead less
Multidimensional Coherent Spectroscopy of Strongly Correlated Materials. By applying new types of spectroscopy, this project aims to address the gaps in our understanding of how remarkable macroscopic properties, such as superconductivity, emerge from the fundamental interactions in strongly correlated electron materials. This project will combine theory and experiment to develop a pathway by which multidimensional coherent spectroscopy can disentangle the competing interactions that make these ....Multidimensional Coherent Spectroscopy of Strongly Correlated Materials. By applying new types of spectroscopy, this project aims to address the gaps in our understanding of how remarkable macroscopic properties, such as superconductivity, emerge from the fundamental interactions in strongly correlated electron materials. This project will combine theory and experiment to develop a pathway by which multidimensional coherent spectroscopy can disentangle the competing interactions that make these materials so complex, but also potentially useful. By delivering an understanding of the interplay between different microscopic processes, the project will make it more feasible to control them. This will allow for the design new controllable quantum materials that can be the basis for future technologies.Read moreRead less
Applications and tests of mesoscopic quantum coherence and entanglement. This project aims to probe the nature of quantum reality at the mesoscopic level. Quantum mechanics predicts strange spooky steering effects. Recent experiments have confirmed such nonlocality between two particles. The project's intended outcome is to provide a theoretical backbone to extend these experiments to larger laboratory- based systems. The objective is theory for experiments enabling spooky action to be quantifie ....Applications and tests of mesoscopic quantum coherence and entanglement. This project aims to probe the nature of quantum reality at the mesoscopic level. Quantum mechanics predicts strange spooky steering effects. Recent experiments have confirmed such nonlocality between two particles. The project's intended outcome is to provide a theoretical backbone to extend these experiments to larger laboratory- based systems. The objective is theory for experiments enabling spooky action to be quantified and quantum paradoxes including the notion of parallel universes to be better understood. Anticipated outcomes are the use of quantum nonlocality to provide secure communication and ultra-sensitive measurement capabilities.Read moreRead less
Advanced framework materials for hydrogen storage applications. This project aims to develop new molecular materials capable of the highly efficient storage of hydrogen gas. Through an innovative interdisciplinary approach that targets the synthesis and detailed characterisation of two classes of molecular material this project expects to generate step-change advances in the understanding of how hydrogen gas uptake relates to the chemical and physical attributes of porous molecular systems. Sign ....Advanced framework materials for hydrogen storage applications. This project aims to develop new molecular materials capable of the highly efficient storage of hydrogen gas. Through an innovative interdisciplinary approach that targets the synthesis and detailed characterisation of two classes of molecular material this project expects to generate step-change advances in the understanding of how hydrogen gas uptake relates to the chemical and physical attributes of porous molecular systems. Significant anticipated outcomes and benefits include the development of new material design approaches that optimise performance across a diverse parameter space, and the generation of advanced new materials worthy of commercial development, spanning small scale mobile to large scale stationary storage applications.Read moreRead less
Polarons in flatland. This project aims to generate new theories of excitons (the solid-state analogue of hydrogen atoms) in charge-doped atomically thin semiconductors. Such theories are urgently needed to describe the response to external probes, such as electric fields, of a range of novel materials that have emerged in recent years. The novelty is to treat the behaviour of semiconductors as a quantum impurity problem, where the excitons become modified by the surrounding electrons to form ne ....Polarons in flatland. This project aims to generate new theories of excitons (the solid-state analogue of hydrogen atoms) in charge-doped atomically thin semiconductors. Such theories are urgently needed to describe the response to external probes, such as electric fields, of a range of novel materials that have emerged in recent years. The novelty is to treat the behaviour of semiconductors as a quantum impurity problem, where the excitons become modified by the surrounding electrons to form new types of particles. A greater understanding of the impurity problem in 2D materials would ultimately facilitate their use in emerging technologies that combine electronics with photonics, for use in ultra-low-power devices such as photodectectors, LEDs, and lasers.Read moreRead less